Spin-Flop Transition and Magnetocaloric Effect through Disconnected Magnetic Blocks in CoIII/CoIV Oxybromides

Spin-Flop Transition and Magnetocaloric Effect through Disconnected Magnetic Blocks in CoIII/CoIV Oxybromides

Magnetocaloric effect in quantum spin-s chains

We compute the entropy of antiferromagnetic quantum spin-s chains in an external magnetic field using exact diagonalization and Quantum Monte Carlo simulations. The magnetocaloric effect, i.e., temperature variations during adiabatic field changes, can be derived from the isentropes. First, we focus on the example of the spin-s = 1 chain and show that one can cool by closing the Haldane gap wit...

Tunable magnetocaloric effect in transition metal alloys

The unpredictability of geopolitical tensions and resulting supply chain and pricing instabilities make it imperative to explore rare earth free magnetic materials. As such, we have investigated fully transition metal based "high entropy alloys" in the context of the magnetocaloric effect. We find the NiFeCoCrPdx family exhibits a second order magnetic phase transition whose critical temperatur...

Hydrostatic pressure effect on magnetic phase transition and magnetocaloric effect of metamagnetic TmZn compound

The magnetocaloric effect (MCE) is an intrinsic thermal response of all magnetic solids which has a direct and strong correlation with the corresponding magnetic phase transition. It has been well recognized that the magnetic phase transition can be tuned by adjusting applied pressure. Therefore, we perform the high hydrostatic pressure magnetization measurements (up to 1.4 GPa) on a recently r...

Ultrafast Magnetism of a Ferrimagnet across the Spin-Flop Transition in High Magnetic Fields.

We show that applying magnetic fields up to 30 T has a dramatic effect on the ultrafast spin dynamics in ferrimagnetic GdFeCo. Upon increasing the field beyond a critical value, the dynamics induced by a femtosecond laser excitation strongly increases in amplitude and slows down significantly. Such a change in spin response is explained by different dynamics of the Gd and FeCo magnetic sublatti...